Re: SYTO red and HOECHST or DAPI

From: Howard Shapiro (hms@shapirolab.com)
Date: Wed Jun 06 2001 - 20:33:13 EST


Elena Soriano wrote-

>My intention is to use SYTO red for RNA specific staining like I use
>Pyronine- Y. Does anyone knows if this possible?
>
>When I stain the DNA with Hoechst or DAPI (selective for DNA), the
>Pyronine-Y finds no place in these molecules, and therefore binds only to
>the RNA, wich is then the only nucleic acid that has free binding points.
>
>-> Could I block the DNA with Hoechst or DAPI and then stain with SYTO red
>to detect the RNA?
>
>Would SYTO red still find free binding points when the DNA is allready
>stained with one of these DNA selective fluorochromes?

This is an interesting question.  Pyronin Y is believed to stain
double-stranded (e.g., ribosomal) RNA, and its structural similarity to
acridine orange suggests an intercalative binding mechanism for the
staining.  As Ingrid Schmid et al have shown, pyronin Y also stains DNA;
again, one would presume binding to be intercalative.  However, the
DNA-specific dyes which demonstrably block pyronin Y staining of DNA (the
list includes the Hoechst dyes and DAPI, which are fluorescent, and methyl
green, which is not, at least when excited with blue-green or green light)
are outer groove binders which bind to to A-T triplets.  I haven't seen
anything on the molecular mechanism of the blocking; one possibility is
that the outer groove binding of the DNA-specific stain unwinds the double
helix somewhat, preventing intercalative binding of tricyclic dyes such as
pyronin Y.

The SYTO dyes are said to bind intercalatively to both double-stranded DNA
and double-stranded RNA; their fluorescence enhancement on binding is
substantially larger than the fluorescence enhancement of Hoechst dyes or
DAPI (and even higher than pyronin fluorescence enhancement, which is
minimal).  Whether the DNA-specific dyes would block binding and
fluorescence of SYTO dyes is not clear a priori; you'd have to do the
experiment.  A good test subject would be a stimulated lymphocyte culture;
the idea would be to compare 2-dimensional displays of Hoechst/pyronin- and
Hoechst/SYTO red-stained cells.  Lymphoblasts in culture typically don't
have the G0 (or G1q) subpopulation, but you could compare them to
peripheral blood lymphocytes, the great majority of which are normally in G1q.

A few years back, we tried several styryl and cyanine dyes which stain both
DNA and RNA in combination with Hoechst dyes; we did not find the blocking
effect (unpublished).  The cyanine dyes we looked at were probably similar
to SYTO red in structure, but it's still worthwhile doing the
experiment.  In theory, a mixture of two dyes which stain both DNA and RNA,
but with different affinities (one more DNA-specific, the other more
RNA-specific), could be used to determine DNA and RNA content using the
same mathematics used for immunofluorescence compensation; I don't think
anybody has actually done this yet.  If I get around to playing with any of
this in the next few months, I'll probably put it in the 4th Edition of
Practical Flow Cytometry.

-Howard



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