Re: SEPARATIONS PROBLEM: TINY GLASS SPHERES

From: Mark Kukuruga (kukuru@med.umich.edu)
Date: Wed Mar 28 2001 - 12:42:35 EST


Elaine,
Consider side scatter as a selection parameter . . . the AU particles should have a
high SS signal to start, and the addition of material may increase (hopefully) in a
proportional manner.  I can't predict what the distribution will look like, and a (very)
quick search revealed no references.  But I can recall this type of analysis being done
(in the "early days" of flow . . .).  Certainly, it parallels the development/analysis
of the beads we run all the time.
Regarding their size . . .  100 nm approaches the threshold of resolution for most
flow cytometers.  I've run 50 nm particles, but had to rely on fluorescence to detect
these initially.  I found 100 nm particles with -out fluorescence, but it's not easy.
Uniformity is key . . . if your particles vary dramatically, you'll have a harder time
making sense of the data.  Also, smaller particles behave erratically in a fluid stream,
not as predictably as do "larger" particles, like cells.  This makes sorting even more
difficult, but I'd worry about that later.
Going back to the reference of bead development . . . can you modify the layering
material to include a fluorescent dye? You could then monitor the accumulation be
fluorescence increase.
Finally, considering your need to separate these by size . . . in my very cursory
search, I did see a reference for electrophoretic separation of microparticles - -
perhaps that's a way to go.
MAK.


--
Mark A. KuKuruga, Managing Director
University of Michigan Flow Core
7416 CCGC 0946
(734) 647-3216, fax (734) 936-7376
kukuru@umich.edu


>>> Elaine Kunze <mek4@psu.edu> 03/26/01 03:43PM >>>

I am sending this again because the replies I have gotten are all talking
about LARGE particles.  These are tiny, little 100 nanometer particles.
Now, are there any suggestions?

What I sent originally:

One of my reseachers is  having difficulty separating a mixture of glass
spheres and glass-coated, colloidal Au, core-shell particles.  The free
glass spheres nucleate and grow under the reaction conditions for the
growth of the core-shell particle.  The typical ratio of the free glass
spheres to core-shell structures is ~100:1.  The size of the core-shell
particles is between 100-115 nm in diameter.  The free silica particles are
only slightly smaller in diameter (by about 5-10 nm).
He has tried gradient separation and gradient centrifugation with a high MW
dextran and low MW PEG, but has not come across appropriate conditions for
separation.  He is currently exploring the use of flow cytometry.  Any
suggestions are greatly appreciated?
****************************************************************************
	Elaine Kunze
	Flow Cytometry.....Image Analysis...
	Life Sciences Consortium
	8B Althouse Laboratory	(814-863-2762)
	Penn State University
	University Park, PA 16802



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